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Journal Articles

Measurement of 107-MeV proton-induced double-differential neutron yields for iron for research and development of accelerator-driven systems

Iwamoto, Hiroki; Nakano, Keita; Meigo, Shinichiro; Satoh, Daiki; Iwamoto, Yosuke; Ishi, Yoshihiro*; Uesugi, Tomonori*; Kuriyama, Yasutoshi*; Yashima, Hiroshi*; Nishio, Katsuhisa; et al.

JAEA-Conf 2022-001, p.129 - 133, 2022/11

For accurate prediction of neutronic characteristics for accelerator-driven systems (ADS) and a source term of spallation neutrons for reactor physics experiments for the ADS at Kyoto University Critical Assembly (KUCA), we have launched an experimental program to measure nuclear data on ADS using the Fixed Field Alternating Gradient (FFAG) accelerator at Kyoto University. As part of this program, the proton-induced double-differential thick-target neutron-yields (TTNYs) and cross-sections (DDXs) for iron have been measured with the time-of-flight (TOF) method. For each measurement, the target was installed in a vacuum chamber on the beamline and bombarded with 107-MeV proton beams accelerated from the FFAG accelerator. Neutrons produced from the targets were detected with stacked, small-sized neutron detectors composed of the NE213 liquid organic scintillators and photomultiplier tubes, which were connected to a multi-channel digitizer mounted with a field-programmable gate array (FPGA), for several angles from the incident beam direction. The TOF spectra were obtained from the detected signals and the FFAG kicker magnet's logic signals, where gamma-ray events were eliminated by pulse shape discrimination applying the gate integration method to the FPGA. Finally, the TTNYs and DDXs were obtained from the TOF spectra by relativistic kinematics.

Journal Articles

Measurement of thick target neutron yield at 180$$^{circ}$$ for a mercury target induced by 3-GeV protons

Matsuda, Hiroki; Iwamoto, Hiroki; Meigo, Shinichiro; Takeshita, Hayato*; Maekawa, Fujio

Nuclear Instruments and Methods in Physics Research B, 483, p.33 - 40, 2020/11

 Times Cited Count:3 Percentile:36.4(Instruments & Instrumentation)

A thick target neutron yield for a mercury target at an angle of 180$$^{circ}$$ from the incident beam direction is measured with the time-of-flight method using a 3-GeV proton beam at the Japan Proton Accelerator Research Complex (J-PARC). Comparing the experimental result with a Monte Carlo particle transport simulation by the Particle and Heavy Ion Transport code System (PHITS) shows that there are apparent discrepancies. We find that this trend is consistent with an experimental result of neutron-induced re- action rates obtained using indium and niobium activation foils. Comparing proton-induced neutron-production double-differential cross-sections for a lead target at backward directions between the PHITS calculation and experimental data suggests that the dis- crepancies for our experiments would be linked to the neutron production calculation around 3 GeV by the PHITS spallation model and/or the calculation of nonelastic cross-sections around 3 GeV in the particle transport simulation.

Journal Articles

Continuous and discontinuous yielding behaviors in ferrite-cementite steels

Wang, Y.*; Tomota, Yo*; Omura, Takahito*; Gong, W.*; Harjo, S.; Tanaka, Masahiko*

Acta Materialia, 196, p.565 - 575, 2020/09

 Times Cited Count:31 Percentile:90.48(Materials Science, Multidisciplinary)

Journal Articles

Thick target neutron yields from 100- and 230-MeV/nucleon helium ions bombarding water, PMMA, and iron

Tsai, P.-E.; Heilbronn, L. H.*; Lai, B.-L.*; Iwata, Yoshiyuki*; Murakami, Takeshi*; Sheu, R.-J.*

Nuclear Instruments and Methods in Physics Research B, 449, p.62 - 70, 2019/06

 Times Cited Count:3 Percentile:32.64(Instruments & Instrumentation)

The secondary neutrons produced from 100- and 230-MeV/nucleon He ions, respectively, stopping in the thick iron, PMMA and water targets are measured by the time of flight method combined with the pulse shape discrimination of liquid scintillators. The experimental data show that the secondary neutrons were contributed from breakup of projectiles, emission from overlap regions of projectile nuclei and target nuclei, and evaporation of projectiles and target nuclei. The measured double-differential thick target neutron yields, angular distributions, and total neutron yields per ion, were benchmarked by the PHITS, FLUKA, and MCNP model calculations. The default models in these codes agree the experimental data well at intermediate-to-large angles in the low-to-intermediate energy range. However, the physics models implemented in PHITS need further improvement for some particular nuclear interaction mechanisms, and this work can be an importance reference for future model development.

Journal Articles

Experimental determination of the photooxidation of aqueous I$$^{-}$$ as a source of atmospheric I$$_{2}$$

Watanabe, Kosuke*; Matsuda, Shohei; Cuevas, C. A.*; Saiz-Lopez, A.*; Yabushita, Akihiro*; Nakano, Yukio*

ACS Earth and Space Chemistry (Internet), 3(4), p.669 - 679, 2019/04

 Times Cited Count:8 Percentile:43.59(Chemistry, Multidisciplinary)

The photooxidation of aqueous iodide ions (I$$^{-}$$$$_{(aq)}$$) at sea surface results in the emission of gaseous iodine molecules (I$$_{2}$$$$_{(g)}$$) into the atmosphere. It plays a certain role in the transport of iodine from ocean to the atmosphere in the natural cycle of iodine. In this study, we determined the photooxidation parameters, the molar absorption coefficient ($$varepsilon$$$$_{iodide}$$($$lambda$$)) and the photooxidative quantum yields ($$Phi$$$$_{iodide}$$($$lambda$$)) of I$$^{-}$$$$_{(aq)}$$, in the range of 290-500 nm. Through the investigation of the influence of pH and dissolved oxygen (DO) on $$Phi$$$$_{iodide}$$($$lambda$$), the subsequent emission rates of I$$_{2}$$$$_{(g)}$$ following the photooxidation of I$$^{-}$$$$_{(aq)}$$ in deionized water solution (pH 5.6, DO 7.8 mg L$$^{-1}$$) and artificial seawater solution (pH 8.0, DO 7.0 mg L$$^{-1}$$) were estimated. A global chemistry-climate model employed herein to assess the I$$_{2}$$$$_{(g)}$$ ocean emission on a global scale indicated that the photooxidation of I$$^{-}$$$$_{(aq)}$$ by solar light can enhance the atmospheric iodine budget by up to $$sim$$8% over some oceanic regions.

Journal Articles

Influence of temperature histories during reactor startup periods on microstructural evolution and mechanical properties of austenitic stainless steel irradiated with neutrons

Kasahara, Shigeki; Kitsunai, Yuji*; Chimi, Yasuhiro; Chatani, Kazuhiro*; Koshiishi, Masato*; Nishiyama, Yutaka

Journal of Nuclear Materials, 480, p.386 - 392, 2016/11

 Times Cited Count:0 Percentile:0.01(Materials Science, Multidisciplinary)

This paper addresses influence of two different temperature profiles during startup periods in the Japan Materials Testing Reactor and a boiling water reactor upon microstructural evolution and mechanical properties of austenitic stainless steel irradiated with neutrons to about 1 dpa and 3 dpa. Tensile tests at 290$$^{circ}$$C and Vickers hardness tests at room temperature were carried out, and their microstructures were observed by FEG-TEM. Influence of difference in the temperature profiles was observed obviously in interstitial cluster formation, in particular, growth of Frank loops. The influence was also found certainly in loss of strain hardening capacity and ductility, although the influence on the yield strength and the Vickers hardness was not clearly observed. As a result, Frank loops, which were observed in austenitic stainless steel irradiated at doses of 1 dpa or more, were considered to contribute to deformation of the austenitic stainless steel.

Journal Articles

Impact of PHITS spallation models on the neutronics design of an accelerator-driven system

Iwamoto, Hiroki; Nishihara, Kenji; Iwamoto, Yosuke; Hashimoto, Shintaro; Matsuda, Norihiro; Sato, Tatsuhiko; Harada, Masahide; Maekawa, Fujio

Journal of Nuclear Science and Technology, 53(10), p.1585 - 1594, 2016/10

 Times Cited Count:18 Percentile:85.7(Nuclear Science & Technology)

Journal Articles

Measurement of neutron spectra produced in the forward direction from thick graphite, Al, Fe and Pb targets bombarded by 350 MeV protons

Iwamoto, Yosuke; Taniguchi, Shingo*; Nakao, Noriaki*; Itoga, Toshio*; Nakamura, Takashi*; Nakane, Yoshihiro; Nakashima, Hiroshi; Satoh, Daiki; Yashima, Hiroshi*; Yamakawa, Hiroshi*; et al.

Nuclear Instruments and Methods in Physics Research A, 562(2), p.789 - 792, 2006/06

 Times Cited Count:6 Percentile:43.85(Instruments & Instrumentation)

Neutron energy spectra produced from thick targets play an important role in validation of calculation codes that are employed in the design of spallation neutron sources and the shielding design of accelerator facilities. However, appropriate experimental data were scarce in the forward direction for the incident energy higher than 100 MeV. In this study, neutron spectra at 0 degree from thick targets bombarded with 350 MeV protons were measured by the time-of-flight technique using an NE213. The targets used were graphite, Al, Fe and Pb and their thicknesses were chosen to be a little thicker than the stopping lengths. The experiment was carried out at the TOF course of the RCNP (Research Center of Nuclear Physics) ring cyclotron, Osaka University. The flight path length between center of the target and of an NE213 were 11.4 m for the measurement of low energy neutrons and 95 m for high energy neutrons. The experimental data are compared with the calculated results by using the Monte Carlo transport codes, such as MCNPX and PHITS codes.

Journal Articles

Corrections to the $$^{148}$$Nd method of evaluation of burnup for the PIE samples from Mihama-3 and Genkai-1 reactors

Suyama, Kenya; Mochizuki, Hiroki*

Annals of Nuclear Energy, 33(4), p.335 - 342, 2006/03

 Times Cited Count:8 Percentile:49.58(Nuclear Science & Technology)

The value of the burnup is one of the most important parameters of samples taken by post irradiation examination (PIE). In this study, concerning the PIE data from Mihama-3 and Genkai-1 PWRs, which were taken at the Japan Atomic Energy Research Institute, the burnup values of the PIE samples were re-evaluated and the PIE data are re-analyzed using SWAT and SWAT2 code systems with JENDL-3.3 library. This analysis concludes that the burnup values of samples from Mihama-3 and Genkai-1 PWRs should be corrected of 2-3%. The effect of re-evaluation of the burnup value on the neutron multiplication factor is approximately 1% for PIE samples having the burnup of larger than 30 GWd/t. Comparison between calculation results using a single pin cell model and an assembly model is carried out. Because the both results agreed within a few percents, we concluded that the single pin cell model is suitable for the analysis of PIE samples and the underestimation of plutonium isotopes does not result from the geometry model.

Journal Articles

Derivation of simple evaluation method for thermal shock damage on accelerator materials caused by out-of-control beam pulses and its application to J-PARC

Takei, Hayanori; Kobayashi, Hitoshi*

Journal of Nuclear Science and Technology, 42(12), p.1032 - 1039, 2005/12

 Times Cited Count:3 Percentile:24.22(Nuclear Science & Technology)

In high-intensity proton accelerator facilities, a failure of an electromagnet that steers beam pulses may result in thermal shock damage on the accelerator component by injecting an out-of-control pulse. It is important that a Machine Protection System (MPS) is appropriately designed to prevent this damage in the facilities such as Japan Proton Accelerator Research Complex (J-PARC). In this study, the simple evaluation method for the allowable injection time before the operation of the MPS was derived from the relation between the thermal stress and the yield stress of materials.The derived evaluation method was then applied to J-PARC. The allowable injection time for each component ranged from 0.1 to 70 $$mu$$s.

Journal Articles

Neutron diagnostics for the energetic ion transport analysis

Nishitani, Takeo; Osakabe, Masaki*; Shinohara, Koji; Ishikawa, Masao

Purazuma, Kaku Yugo Gakkai-Shi, 80(10), p.860 - 869, 2004/10

no abstracts in English

Journal Articles

Validation of minor actinide cross sections by studying samples irradiated for 492 days at the dounreay prototype fast reactor, 2; Burnup calculations

Tsujimoto, Kazufumi; Kono, Nobuaki; Shinohara, Nobuo; Sakurai, Takeshi; Nakahara, Yoshinori; Mukaiyama, Takehiko; Raman, S.*

Nuclear Science and Engineering, 144(2), p.129 - 141, 2003/06

To evaluate neutron cross-section data of minor actinides, separated actinide samples and dosimetry samples were irradiated at the Dounreay Prototype Fast Reactor for 492 effective full power days. Based on the burnup calculations of major actinide and dosimetry samples, the neutron flux distribution and the flux level were adjusted at the locations where minor actinide samples were irradiated. The burnup calculations were carried out for minor actinides using the determined flux distribution and flux level. This paper discusses the burnup calculations and the validation of minor actinide cross-section data in evaluated nuclear data libraries. We find that we can obtain reliable FIMA (fission per initial metallic atom) values by using the $$^{148}$$Nd method except that the uncertainties in the FIMA values are large for $$^{234}$$U, $$^{238}$$Pu, Am isotopes, and Cm isotopes because the $$^{148}$$Nd yields are known poorly for these isotopes and are probably overestimated. For these isotopes, measurements to improve the fission-yield data are needed. We also find that, in general, the JENDL-3.2 nuclear data for the minor actinides are adequate for the conceptual design study of transmutation systems. But, there are some nuclides (especially $$^{238}$$Pu and $$^{242}$$Pu) for which new measurements are needed particulary if the minor actinides constitute a major part of the nuclear fuel.

Journal Articles

Validation of minor actinide cross sections by studying samples irradiated for 492 days at the dounreay prototype fast reactor, 2; Burnup calculations

Tsujimoto, Kazufumi; Kono, Nobuaki; Shinohara, Nobuo; Sakurai, Takeshi; Nakahara, Yoshinori; Mukaiyama, Takehiko*; Raman, S.*

Nuclear Science and Engineering, 144(2), p.129 - 141, 2003/06

 Times Cited Count:11 Percentile:59.38(Nuclear Science & Technology)

no abstracts in English

JAEA Reports

A Systematics of fission product mass yields with 5 gaussian functions

Katakura, Junichi

JAERI-Research 2003-004, 19 Pages, 2003/03

JAERI-Research-2003-004.pdf:0.76MB

no abstracts in English

Journal Articles

Shielding experiments and analyses on proton accelerator facility at TIARA

Nakashima, Hiroshi; Sakamoto, Yukio*; Tanaka, Shunichi; Tanaka, Susumu; Baba, Mamoru*; Nakamura, Takashi*; Hirayama, Hideo*; Shin, Kazuo*; JAERI-Universities Collaboration Working Group for Accelerator Shielding Study

Proceedings of 6th International Meeting on Nuclear Applications of Accelerator Technology (AccApp '03), p.959 - 968, 2003/00

In order to validate shielding design methods on proton accelerator facilities, a series of shielding experiments in several tens of MeV energy region were carried out at the Takasaki Ion Accelerators for Advanced Radiation Application (TIARA) of Japan Atomic Energy Research Institute (JAERI). The experiments include thick target neutron yield (TTY) measurements by charged particles, deep penetration experiments on concrete, steel and polyethylene shields using p-Li monoenergetic neutron source and radiation streaming experiment at a labyrinth of TIARA using p-Cu white neutron source. These experimental results are compared with calculation results with some high-energy particle transport codes such as MCNPX and NMTC/JAERI. The TTY measurements were analyzed by a code developed by Shin with a moving source model, and the streaming experiment was also analyzed by the DUCT-III code based on Shin's equation. This paper reviews the experimental results and the analyses on the results.

Journal Articles

Adjustment of total delayed neutron yields of $$^{235}$$U, $$^{238}$$U and $$^{239}$$Pu by using results of in-pile measurements of effective delayed neutron fraction

Sakurai, Takeshi; Okajima, Shigeaki

Proceedings of International Conference on the New Frontiers of Nuclear Technology; Reactor Physics, Safety and High-Performance Computing (PHYSOR 2002) (CD-ROM), 12 Pages, 2002/10

The cross section adjustment method was applied to total delayed neutron yields of $$^{235}$$U, $$^{238}$$U and $$^{239}$$Pu of the JENDL-3.2 file by using experimental results of effective delayed neutron fraction $$beta_{eff}$$ at six cores built in two fast critical facilities of the MASURCA and FCA and a thermal critical facility of the TCA to improve these yields. The adjustment was carried out on the yields given at several incident neutron energy points in the file. Furthermore, to validate these adjusted delayed neutron yields, analyses were performed for the $$beta_{eff}$$ experiments at ZPR fast critical facility. These adjusted yields brought a reduction of uncertainty of calculated $$beta_{eff}$$ and an improvement in agreement of $$beta_{eff}$$ between experiment and calculation.

Journal Articles

Evaluation of Delayed Neutron Data for JENDL-3.3

Yoshida, Tadashi*; Okajima, Shigeaki; Sakurai, Takeshi; Nakajima, Ken; Yamane, Tsuyoshi; Katakura, Junichi; Tahara, Yoshihisa*; Zukeran, Atsushi*; Oyamatsu, Kazuhiro*; Osawa, Takaaki*; et al.

Journal of Nuclear Science and Technology, 39(Suppl.2), p.136 - 139, 2002/08

no abstracts in English

Journal Articles

Photofission of $$^{209}$$Bi at intermediate energies

Haba, Hiromitsu; Kasaoka, Makoto*; Igarashi, Manabu*; Washiyama, Koshin*; Matsumura, Hiroshi*; Oura, Yasuji*; Shibata, Seiichi*; Sakamoto, Ko*; Furukawa, Michiaki*; Fujiwara, Ichiro*

Radiochimica Acta, 90(7), p.371 - 382, 2002/08

 Times Cited Count:2 Percentile:17.03(Chemistry, Inorganic & Nuclear)

The reaction yields of 63 radionuclides with the mass number A = 56-135 produced in the photofission of $$^{209}$$Bi by bremsstrahlung of end-point energies (E$$_{0}$$) from 450 to 1100 MeV have been measured using a catcher foil technique. The charge distribution was well reproduced by a Gaussian function with the most probable charge (Z$$_{p}$$) expressed by Z$$_{p}$$ = RA + S, and with the A-independent FWHME$$_{CD}$$. The charge distribution parameters R, S and FWHM$$_{CD}$$ were independent of E$$_{0}$$ above 600 MeV. The weighted mean values at E$$_{0}$$ $$geq$$ 600 MeV were R = 0.421 $$pm$$ 0.001, S = 0.6 $$pm$$ 0.1 and FWHM$$_{CD}$$ = 2.1 $$pm$$ 0.1 charge unit (c.u.). Based on the charge distribution parameters, the symmetric mass yield distributions with the most probable mass A$$_{p}$$ of 96 $$pm$$ 1 mass unit (m.u.) and the width FWHM$$_{MD}$$ of 33 $$pm$$ 1 m.u. were also obtained. The characteristics of the charge and mass yield distributions are discussed by referring to those for $$^{197}$$Au based on the results of calculations using PICA3/GEM.

JAEA Reports

Design of ex-vessel neutron monitor for ITER

Nishitani, Takeo; Iguchi, Tetsuo*; Ebisawa, Katsuyuki*; Yamauchi, Michinori*; Walker, C.*; Kasai, Satoshi

JAERI-Tech 2002-062, 39 Pages, 2002/07

JAERI-Tech-2002-062.pdf:1.65MB

no abstracts in English

Journal Articles

Adjustment of total delayed neutron yields of $$^{235}$$U, $$^{238}$$U and $$^{239}$$Pu in JENDL-3.2 using benchmark experiments on effective delayed neutron fraction $$beta_{eff}$$

Sakurai, Takeshi; Okajima, Shigeaki

Journal of Nuclear Science and Technology, 39(1), p.19 - 30, 2002/01

 Times Cited Count:6 Percentile:39.54(Nuclear Science & Technology)

The cross section adjustment method was applied to total delayed neutron yields of $$^{235}$$U, $$^{238}$$U and $$^{239}$$Pu of the JENDL-3.2 file by using experimental results of effective delayed neutron fraction $$beta_{eff}$$ at six cores built in two fast critical facilities of the MASURCA and FCA and a thermal critical facility of the TCA to improve these yields. The adjustment was carried out on the yields given at several incident neutron energy points in the file. After the adjustment, the yield of $$^{238}$$U was almost uniformly decreased by about 3% below 7 MeV. The yield of $$^{239}$$Pu was increased by 2.6% and that of $$^{235}$$U was decreased by 0.9% at the thermal energy point, while the change of yield was less than 0.3% at the other energy points for these nuclides. By using these adjusted yields, the uncertainty of calculated $$beta_{eff}$$ was reduced and the agreement of $$beta_{eff}$$ between experiment and calculation was improved.

73 (Records 1-20 displayed on this page)